Cochran, J. K., D. J. Hirschberg, H. D. Livingston, K. O. Buesseler, and R. M. Key, 1995: Natural and anthropogenic radionuclide distributions in the Nansen Basin, Arctic Ocean: Scavenging rates and circulation timescales. Deep-Sea Research, Part II, 42(6), 1495-1517.
Abstract: Determination of the naturally occurring radionuclides
232Th, 230Th,
228Th and 210Pb,
and the anthropogenic radionuclides 241Am,
239,240Pu, 134Cs
and 137Cs in water samples collected across
the Nansen Basin from the Barents Sea slope to the Gakkel Ridge provides
tracers with which to characterize both scavenging rates and circulation
timescales in this portion of the Arctic Ocean. Large volume water samples
( ~ 1500 l) were filtered in situ to separate particulate (>
0.5 µm) and dissolved Th isotopes and 241Am.
Thorium-230 displays increases in both particulate and dissolved activities
with depth, with dissolved 230Th greater
and particulate 230Th lower in the deep
central Nansen Basin than at the Barents Sea slope. Dissolved 228Th
activities also are greater relative to 228Ra,
in the central basin. Residence times for Th relative to removal from solution
onto particles are ~ 1 year in surface water, ~ 10 years in deep water
adjacent to the Barents Sea slope, and ~ 20 years in the Eurasian Basin
Deep Water. Lead-210 in the central basin deep water also has a residence
time of ~ 20 years with respect to its removal from the water column. This
texture of scavenging is reflected in distributions of the particle-reactive
anthropogenic radionuclide 241Am, which
shows higher activities relative to Pu in the central Nansen Basin than
at the Barents Sea slope.
Distributions of 137Cs show more rapid
mixing at the basin margins (Barents Sea slope in the south, Gakkel Ridge
in the north) than in the basin interior. Cesium-137 is mixed throughout
the water column adjacent to the Barents Sea slope and is present in low
but detectable activities in the Eurasian Basin Deep Water in the central
basin. At the time of sampling (1987) the surface water at all stations
had been labeled with 134Cs released in
the 1986 accident at the Chernobyl nuclear power station. In the ~ 1 year
since the introduction of Chernobyl 134Cs
to the Nansen Basin, it had been mixed to depths of ~ 800 m at the Barents
Sea Slope and to ~ 300 m in the central basin. "Pre-Chernobyl"
inventories of 137Cs (as well as 239,
240Pu) are 10 times those expected from global atmospheric
fallout from nuclear weapons testing and are derived principally from releases
from the Sellafield, U.K., nuclear fuel reprocessing facility on the Irish
Sea. Based on the sources of 137Cs to the
Nansen Basin, mixing time scales are 9 - 18 years for the upper water column
(to 1500 m) and ~ 40 years for the deep water. These mixing time scales,
combined with more rapid scavenging at the basin margin relative to the
central basin, produce residence times of particle-reactive radionuclides
in the Nansen Basin comparable to other open ocean areas (e.g., north-west
Atlantic) despite the presence of permanent ice cover and long periods
of low-light levels that limit productivity in the Arctic.